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We generate self-phase-stabilized pulses by difference-frequency generation of a hollow-fibre broadened supercontinuum followed by two-stage optical parametric amplification. This system allows the production of broadband pulses widely tuneable in the near-IR wavelength region. Energies up to 0.2 mJ with 15 fs pulse width are demonstrated. These characteristics make this source suitable as a driver for attosecond pulse generation. [ABSTRACT FROM AUTHOR]

We demonstrate the complete reconstruction of the electric field of visible–infrared pulses with energy as low as a few tens of nanojoules. The technique allows for the reconstruction of the instantaneous electric field vector direction and magnitude, thus giving access to the characterization of pulses with an arbitrary time-dependent polarization state. The technique combines extreme ultraviolet interferometry with the generation of isolated attosecond pulses. [ABSTRACT FROM AUTHOR]

The coherent interaction with ultrashort light pulses is a powerful strategy for monitoring and controlling the dynamics of wave packets in all states of matter. As light presents an oscillation period of a few femtoseconds (T = 2.6 fs in the near infrared spectral range), an external optical field can induce changes in a medium on the sub-cycle timescale, i.e. in a few hundred attoseconds. In this work, we resolve the dynamics of autoionizing states on the femtosecond timescale and observe the sub-cycle evolution of a coherent electronic wave packet in a diatomic molecule, exploiting a tunable ultrashort extreme ultraviolet pulse and a synchronized infrared field. The experimental observations are based on measuring the variations of the extreme ultraviolet radiation transmitted through the molecular gas. The different mechanisms contributing to the wave packet dynamics are investigated through theoretical simulations and a simple three level model. The method is general and can be extended to the investigation of more complex systems. [ABSTRACT FROM AUTHOR]

We demonstrate the generation of broadband extreme ultraviolet (XUV) continua by high order harmonic generation in neon using carrier-envelope phase (CEP) stabilized, few-cycle pulses with a time-dependent polarization. The XUV spectra can support isolated attosecond pulses with a duration of about 50 as, opening the possibility of achieving time resolution close to the atomic unit of time. A theoretical model that calculates the spectral and temporal characteristics of the XUV radiation emitted by a single atom is used to interpret the CEP dependence of the harmonic structures. [ABSTRACT FROM AUTHOR]