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A general method for rotational microwave spectroscopy and control of polar molecular ions via direct microwave addressing is considered. Our method makes use of spatially varying ac Stark shifts, induced by far off-resonant, focused laser beams to achieve an effective coupling between the rotational state of a molecular ion and the electronic state of an atomic ion. In this setting, the atomic ion is used for read-out of the molecular ion state, in a manner analogous to quantum logic spectroscopy based on Raman transitions. In addition to high-precision spectroscopy, this setting allows for rotational ground state cooling, and can be considered as a candidate for the quantum information processing with polar molecular ions. All elements of our proposal can be realized with currently available technology. [ABSTRACT FROM AUTHOR]

We report on the loading of large ion Coulomb crystals into a linear Paul trap incorporating a high-finesse optical cavity (ℱ∼3000). We show that, even though the 3-mm diameter dielectric cavity mirrors are placed between the trap electrodes and separated by only 12 mm, it is possible to produce in situ ion Coulomb crystals containing more than 105 calcium ions of various isotopes and with lengths of up to several millimeters along the cavity axis. We show that the number of ions inside the cavity mode is, in principle, high enough to achieve strong collective coupling between the ion Coulomb crystal and the cavity field. The results thus represent an important step towards ion trap based Cavity Quantum ElectroDynamics (CQED) experiments using cold ion Coulomb crystals. [ABSTRACT FROM AUTHOR]

An experimental demonstration of a novel all-optical technique for loading ion traps, which has particular application to microtrap architectures, is presented. The technique is based on photoionisation of an atomic beam created by pulsed laser ablation of a calcium target, and provides improved temporal control compared to traditional trap loading methods. Ion loading rates as high as 125 ions per second have so far been observed. Also described are observations of trap loading where Rydberg state atoms are photoionised by the ion Doppler cooling laser. [ABSTRACT FROM AUTHOR]