1. Plasmon resonances and plasmon-induced charge transport in linear atomic chains.
- Author
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Zhang, Hong and Yin, Haifeng
- Subjects
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SURFACE plasmon resonance , *CHARGE transfer , *TIME-dependent density functional theory , *ATOMIC units , *CHEMICAL chains , *EXCITATION spectrum , *ELECTRON delocalization - Abstract
In linear hydrogen atomic chains, plasmon resonances and plasmon-induced charge transport are studied by time-dependent density functional theory. For the large linear chain, it is a general phenomenon that, in the longitudinal excitation, there are high-energy resonances and a large low-energy resonance. The energy of the large low-energy resonance conforms to the results calculated by the classical Drude model. In order to explain the formation mechanism of the high-energy resonances, we present a simple harmonic oscillator model. This model may reasonably account for the relationship between low-energy and high-energy resonances, and has a certain degree of universality. As the interatomic distance decreases, the current shows a gradual transition from insulator to metal. The current enhancement mainly depends on the local field enhancement associated with plasmon excitation, and the enhanced electron delocalization effect as a result of the decrease of the interatomic distance. © 2013 Wiley Periodicals, Inc. [ABSTRACT FROM AUTHOR]
- Published
- 2013
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