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• Theoretical model for MF-PV2S aircraft engine gas exchange is established. • Prediction discrepancies of previous models are analyzed. • Modifying model zones and coefficients improve prediction accuracy. • Adaptability to varying conditions of speed, pressure, valve overlap, fuel type. • Model accuracy is validated by tracer gas method experiments. Under the demand of global aviation carbon reduction, the multi-fuel poppet valves two-stroke (MF-PV2S) aircraft engine exhibits advantages such as lower lubricant consumption and the flexibility to high-altitude valve timing adjustment, which position it to play a more significant role in general aviation aircraft and unmanned aerial vehicle propulsion systems. High-altitude gas exchange performance is a critical factor in the thermal efficiency and power characteristics of two-stroke aircraft engines. However, the applicability and accuracy of existing models in predicting the gas exchange process for PV2S engines remain insufficiently discussed. Recognizing discrepancies in the predictions of PV2S gas exchange processes by existing models, a theoretical model applicable to high-altitude gas exchange in an MF-PV2S aircraft engine is established. The modified model adjusts the exhaust composition during the second and third phases of the scavenging process, and a novel model characteristic coefficient, designated as b 3 , is incorporated to signify the proportion of mixed gas in the exhaust gases at a given moment. Moreover, the model characteristic coefficients b 1 and b 2 , are determined with nonlinearity, based on appropriate relationships that account for the characteristics of the PV2S gas exchange process. The model calculates gas exchange characteristics under different operating conditions and fuels, comparing these results with simulations and tracer gas-based experiments. The findings demonstrate that the model successfully captures the characteristics of early appearance and prolonged duration of fresh charge loss during PV2S gas exchange, significantly enhancing the predictive accuracy. Through adjustments of model coefficients based on specific conditions, the model predicts and describes the variation process of PV2S gas exchange performance parameters under different conditions, including various speeds, different intake-exhaust pressure differences at different altitudes, valve overlaps, and fuel types. The maximum relative errors between model predictions and experimental trapping efficiency, delivery ratio and charging efficiency are 2.58 %, 4.33 %, and 3.89 % respectively. The model can be used for rapid and accurate prediction of gas exchange characteristics under different conditions for the MF-PV2S aircraft engine. Also, it serves as an alternative model of three-dimensional simulation models that can be coupled into the one-dimensional thermodynamic cycle simulation. [ABSTRACT FROM AUTHOR]