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• A widely used hydrological model is applied at the national scale to Spain. • Hydrological ecosystem services are evaluated under a business-as-usual land abandonment scenario. • Land abandonment increases water levels in wetter regions and decreases them in drier areas. • The tool can be easily applied to other countries or basins. This research demonstrates the opportunities and challenges for decision-makers in the use of satellite data driven hydrological model such as WaterWorld to assess current hydrological ecosystem services at the national scale and evaluate the impact of land use scenarios for the future. Spain has been selected as a case study in view of the negative consequences for hydrological ecosystem services caused by land abandonment over the last few decades, which, if action is not taken soon, will make Spain the European Union country most affected by this problem in the coming years. The results show that continued land abandonment will exacerbate the already geographically polarised situation of land abandonment of agricultural areas in the north of the country due to their low economic viability, in contrast to intensification of irrigated area in the most arid regions of Spain, leading to an increase in water balances in the already wet areas and a decrease in the arid areas. However, there is much to be gained from restoration of nature in Spain. Beyond the obvious benefits for biodiversity, climate change mitigation and recreation, abandonment of current agricultural land and its return to natural cover will lead to improvements in water quality ecosystem services. This model used, which is easily replicable to other countries given the availability of a user-friendly interface and embedded global data, can help analyse hydrological ecosystem services in any other country in the world. Like all models and measurements, WaterWorld has limitations so results should be viewed critically, but can still contribute to discussions on land management for sustainability, alongside other source of information. [ABSTRACT FROM AUTHOR]