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(Pb0.325Sr0.675)TiO3 (PST) ceramics were prepared by a traditional solid-state reaction technique. The dielectric and enhanced pyroelectric properties of PST ceramics were investigated under a DC bias field. The dielectric permittivity and dielectric loss of PST ceramics at Curie temperature were 2.97 × 10-4 and 0.006 without DC bias field, respectively. With a DC electric field of 0-500 V/mm, the maximum pyroelectric coefficient and the largest figure of merit (Fd) of PST ceramics were obtained, about 60 × 10-8 C cm-2 K-1 and 26 × 10-5 Pa-1/2, respectively. PST ceramics with such superior electric field enhanced pyroelectric properties have the potential for uncooled focal plane array detectors application. [ABSTRACT FROM AUTHOR]