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Rainwater harvesting (RWH) has become a popular water saving and conservation means across the globe. In many cities, a pre-determined rainwater tank size is generally selected without a detail water balance modelling at the location on interest. However, to achieve maximum benefit from a RWH system at a given location, it is desirable to design the system based on the site specific conditions (e.g. local rainfall and loss characteristics) and other relevant design parameters. There have been limited studies on regionalization of RWH system, which can account for the spatial variability in rainfall, loss and water demand characteristics over a given region to provide site-specific design of RWH system. This paper presents a RWH regionalization approach to develop a set of design curves, which assist in the selection of an adequate RWH system at a given location. We use rainfall data from 159 rain gauges across the Greater Sydney region in Australia to develop and test the proposed regionalization approach. It has been found that there is a significant variation in rainfall characteristics across Greater Sydney region and that a common tank size across this region does not present an adequate solution. It has been found that a 5 kL tank can achieve a reliability (i.e. percentage of days the RWH can meet the given demand) of 31–93% for four people depending on the location in the Greater Sydney region and the types of water use. The developed regional design curves could result in increased water savings across Greater Sydney. The proposed regionalization approach can be adapted to other cities across Australia and the world which present a high rainfall gradient. • Water savings by rainwater harvesting at 159 locations in Sydney are evaluated. • Reliability of a rainwater tank is moderately correlated with mean annual rainfall. • A set of design curves is developed for Sydney to enhance rainwater harvesting. [ABSTRACT FROM AUTHOR]