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The effectiveness of national policies for air pollution control has been demonstrated, but the relative effectiveness of short-term emission reduction measures in comparison with national policies has not. Here we show that short-term abatement measures during important international events substantially reduced PM2.5 concentrations, but air quality rebounded to pre-event levels after the measures ceased. Long-term adherence to strict emission reduction policies led to successful decreases of 54% in PM2.5 concentrations in Beijing, and 23% in atmospheric nitrogen deposition in China from 2012 to 2020. Incentivized by "blue skies" type campaigns, economic development and reactive nitrogen pollution are quickly decoupled, showing that a combination of inspiring but aggressive short-term measures and effective but durable long-term policies delivers sustainable air quality improvement. However, increased ammonia concentrations, transboundary pollutant flows, and the complexity to achieving reduction targets under climate change scenarios, underscore the need for the synergistic control of multiple pollutants and inter-regional action. In response to the rebound of air pollution during large events in China, the authors propose that a combination of ambitious short-term measures and enduring long-term pollution control policies is a sustainable solution for improving air quality. [ABSTRACT FROM AUTHOR]

Currently, air pollution is primarily characterized by PM 2.5 and O 3. Therefore, the co-control of PM 2.5 and O 3 has become an important task of atmosphere pollution prevention and control in China. However, few studies have been conducted on the emissions from vapor recovery and processes, which is an important source of VOCs. This paper analyzed the VOC emissions of three vapor process technologies in service stations and first proposed key pollutants for priority control based on the coordinated reactivity of O 3 and SOA. The concentration of VOCs emitted from the vapor processor was 3.14–9.95 g m−3, compared to 631.2–717.8 g m−3 for uncontrolled vapor. Alkanes, alkenes, and halocarbons accounted for a high proportion of the vapor both before and after control. Among the emissions, i -pentane, n -butane, and i -butane were the most abundant species. Then, the species of OFP and SOAP were calculated through the maximum incremental reactivity (MIR) and fractional aerosol coefficient (FAC). The average source reactivity (SR) value of the VOC emissions from three service stations was 1.9 g g−1, while the OFP ranged from 8.2 to 13.9 g m−3 and SOAP ranged from 0.18 to 0.36 g m−3. By considering the coordinated chemical reactivity of O 3 and SOA, a comprehensive control index (CCI) was proposed for the control of key pollutant species that have multiplier effects on environment. For adsorption, trans -2-butene and p -xylene were the key co-control pollutants, while toluene and trans -2-butene were the most important for membrane and condensation + membrane control. A 50% emission reduction of the top two key species that emission account for 4.3% averagely will reduce O 3 by 18.4% and SOA by 17.9%. [Display omitted] • The organized emissions of VOCs from three vapor processors were studied in service stations. • The species composition of VOCs before and after control were analyzed. • The OFP and SOAP were calculated to evaluate the secondary pollution. • The co-control of key pollutants based on SOA and O 3 has great environmental benefits. [ABSTRACT FROM AUTHOR]